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金属学报  2021, Vol. 57 Issue (3): 283-294    DOI: 10.11900/0412.1961.2020.00165
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含杂质气态CO2输送管道腐蚀研究进展
李玉星1,2(), 刘兴豪1,2, 王财林1,2, 胡其会1,2, 王婧涵1,2, 马宏涛1,2, 张楠1,2
1.中国石油大学(华东) 山东省油气储运安全省级重点实验室 青岛 266580
2.中国石油天然气股份有限公司 油气储运重点实验室 青岛 266580
Research Progress on Corrosion Behavior of Gaseous CO2 Transportation Pipelines Containing Impurities
LI Yuxing1,2(), LIU Xinghao1,2, WANG Cailin1,2, HU Qihui1,2, WANG Jinghan1,2, MA Hongtao1,2, ZHANG Nan1,2
1.Provincial Key Laboratory of Oil and Gas Storage and Transportation Security, China University of Petroleum (East China), Qingdao 266580, China
2.Key Laboratory of Oil & Gas Storage and Transportation, PetroChina Company Limited, Qingdao 266580, China
引用本文:

李玉星, 刘兴豪, 王财林, 胡其会, 王婧涵, 马宏涛, 张楠. 含杂质气态CO2输送管道腐蚀研究进展[J]. 金属学报, 2021, 57(3): 283-294.
Yuxing LI, Xinghao LIU, Cailin WANG, Qihui HU, Jinghan WANG, Hongtao MA, Nan ZHANG. Research Progress on Corrosion Behavior of Gaseous CO2 Transportation Pipelines Containing Impurities[J]. Acta Metall Sin, 2021, 57(3): 283-294.

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摘要: 

气态CO2输送管道是CO2捕集与储存(CCS)过程中的重要一环，含杂质气态CO2输送管道的腐蚀控制对于管道的安全运行尤为重要。本文综述了目前含杂质气态CO2输送管道腐蚀的研究成果，总结了气态CO2输送管道腐蚀的影响因素，阐述了杂质与环境条件对水与CO2的互溶度、管道钢腐蚀行为、腐蚀产物膜特征及腐蚀机理的影响，分析了气态CO2输送管道临界含水量的确定，归纳了适用于气态CO2输送管道的腐蚀预测模型。本文指出当前气态CO2输送管道腐蚀研究亟待解决的科学问题包括：含杂质气态CO2环境中水与CO2互溶度的计算；杂质对气态CO2环境中腐蚀产物膜特征及腐蚀机理的影响；含杂质气态CO2输送管道不发生腐蚀临界含水量的确定；含杂质气态CO2输送管道内腐蚀预测模型的建立。
关键词 ： 气态CO2输送,  腐蚀,  杂质,  互溶度,  临界含水量,  腐蚀预测模型    
Abstract：

Gaseous CO2 transportation pipelines are an important part of carbon capture and storage. Corrosion control of gaseous CO2 transportation pipelines containing impurities is important to the safe operation of pipelines. This paper reviews recent research progress on the corrosion of gaseous CO2 transportation pipelines containing impurities, and the impact factors of gaseous CO2 transportation pipelines are summarized. The influence of pipe impurities and environmental conditions on the mutual solubility of water and CO2, the corrosion behavior of pipelines, the characteristic of corrosion scales, and corrosion mechanism of transportation pipelines are discussed. The determination of critical water content for the corrosion of gaseous CO2 transportation pipelines is analyzed. Predictive corrosion models of gaseous CO2 transportation pipelines are also concluded. For further research on corrosion of gaseous CO2 transportation pipelines containing impurities, the following should be the focal points: the calculation of water and CO2 mutual solubility in gaseous CO2 environments containing impurities, the influence of impurities on corrosion product film characteristics and the corrosion mechanism in a gaseous CO2 environment, the determination of the critical water content of corrosion for gaseous CO2 transportation pipelines containing impurities, and the establishment of inner corrosion prediction models of gaseous CO2 transportation pipelines containing impurities.
Key words： gaseous CO2 transportation    corrosion    impurity    mutual solubility    critical water content    corrosion prediction model
收稿日期: 2020-05-18     
ZTFLH:  TE988  
基金资助:国家科技重大专项项目(2016ZX05016-002);中国石油天然气股份有限公司油气储运重点实验室项目(GDGS-KJZX-2016-JS-379)
作者简介: 李玉星，男，1970年生，教授，博士
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李玉星
刘兴豪
王财林
胡其会
王婧涵
马宏涛
张楠

链接本文:

https://www.ams.org.cn/CN/10.11900/0412.1961.2020.00165      或      https://www.ams.org.cn/CN/Y2021/V57/I3/283

图1  纯CO2相图
Steel

Temperature

oC

Pressure

MPa

H2O contentH2S contentO2 content

Corrosion rate

mm·a-1

Carbon steel[35]402Saturated0.1 MPa00.6223
Carbon steel[35]602Saturated1 MPa00.7706
X65[36]505Saturated000.0186
1000 × 10-60.0435
X65 (Ni-P coating)[36]505Saturated00~0
1000 × 10-60.0093
X65[37]504Saturated00~0.2
6~0.2
X65[38]501Saturated00~1
X65[39]243Saturated001.3077
X70[40]501Saturated000.025
3Cr steel[41]601Saturated000.22
0.950.05 MPa1.36
Low-alloy steel[42]751.2Saturated000.18
Carbon steel[43]603Saturated00~18
5Cr steel[43]~5
13Cr steel[43]~0.2
X65[44,45]354600 × 10-6000.04
60%RH0.05
80%RH0.02
Saturated0.08
表1  近年来气态CO2输送管道腐蚀的研究结果[35~45]
图2  含杂质CO2的相包线[51]
图3  富CO2输送管道最大含水量与压力、温度的关系图[77]
ModelDeveloped byT / ℃P / MPapCO2 / MPa
MinMaxMaxMinMax
LIPUCOR[90]Total2015025-5
KSC[91]IFE515025-5
PREDICT[92,93]InterCorr20200--10
SweetCor[94]Shell5121-0.0217
OLI[95,96]OLI system-50300150-150
表2  适用于气态CO2输送管道的腐蚀速率预测模型[90~96]
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