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Acta Metall Sin  1997, Vol. 33 Issue (5): 543-547    DOI:
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STRUCTURE AND MAGNETIC PROPERTIES OF QUASI-TERNARY TbMn_(6-x)Co_xSn_6 COMPOUNDS
WANG Yingung;CHEN Changpin;WANG Qidong(Zhejiang University; Hangzhou 310027); TANG Ning;YANG Fuming (State Key Laboratory of Magnetism; Institute of Physics; Chinese Academy of Sciences; Beijing 100080)
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WANG Yingung;CHEN Changpin;WANG Qidong(Zhejiang University; Hangzhou 310027); TANG Ning;YANG Fuming (State Key Laboratory of Magnetism; Institute of Physics; Chinese Academy of Sciences; Beijing 100080). STRUCTURE AND MAGNETIC PROPERTIES OF QUASI-TERNARY TbMn_(6-x)Co_xSn_6 COMPOUNDS. Acta Metall Sin, 1997, 33(5): 543-547.

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Abstract  Structure and magnetic properties of quasi-ternary TbMn6-xCoxSn6 compounds with x=0.0, 0.3, 0.6, 0.9, 1.2 and 1.5 have been studied. The structure of TbMn6-xCoxSn6 compounds has not been changed on Co substitution. The substitution of Co for Mn in TbMn6Sn6 results in a monotonous decrease in the lattice constants and the unit-cell volume. The ordering temperature decreases monotonously with increasing Co content. The reorientation temperature decreases with increasing Co content and the reorientation of easy axis magnetization of TbMn6Sn6 disappeared at x=0.6. When x exceeding 0.9 a compensation temperature was observed in the thermal magnetization curve and the compensation temperature increases with increasing Co content. The saturation magnetization at 4.5 K decreases to a minimum at x=0.6 and then increases again.
Key words:  TbMn_(6-x)Co_xSn_6      structure      magnetic phase transition      saturation magnetization     
Received:  18 May 1997     
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