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Acta Metall Sin  2022, Vol. 58 Issue (1): 17-27    DOI: 10.11900/0412.1961.2021.00193
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Research Progress of High-Entropy Alloy Coatings
CUI Hongzhi1,2(), JIANG Di2
1. School of Materials Science and Engineering, Ocean University of China, Qingdao 266100, China
2. School of Materials Science and Engineering, Shandong University of Science and Technology, Qingdao 266590, China
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CUI Hongzhi, JIANG Di. Research Progress of High-Entropy Alloy Coatings. Acta Metall Sin, 2022, 58(1): 17-27.

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Abstract  

Preparing various types of coatings to strengthen the surface of materials is an effective technique to increase the materials' service performance. The qualities of the coatings can be considerably improved based on the service environment by altering their composition and microstructure without impacting the substrate's performance, thereby extending the equipment's service life. Recently, high- entropy alloys (HEAs) and their coatings have been the focus in materials science. The applications in surface engineering have developed rapidly owing to their outstanding strength, toughness, corrosion resistance, and wear resistance. By designing different HEA coatings and developing efficient preparation methods for surface engineering, HEA coatings are expected to be an ideal candidate for surface strengthening of key components suffering from wear, corrosion, and elevated temperature in an extreme environment. In this paper, the latest research results are detailed and the compositions, structures, properties, and wear and corrosion mechanisms of HEA coating from the characters viewpoint, classification, and preparation methods of HEA coatings are summarized. In addition, the issues that must be solved in the surface engineering field and the developing direction in the future were proposed.
Key words:  high-entropy alloy (HEA) coating      wear      corrosion     
Received:  07 May 2021     
ZTFLH:  TG178  
Fund: National Natural Science Foundation of China(51971121);Major-Special Science and Technology Projects in Shandong Province(2019JZZY010303)
About author:  CUI Hongzhi, professor, Tel: (0532)86057929, E-mail: cuihongzhi@ouc.edu.cn
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https://www.ams.org.cn/EN/10.11900/0412.1961.2021.00193     OR     https://www.ams.org.cn/EN/Y2022/V58/I1/17

Coating Process parameter Amorphous content Microhardness Ref.
(atomic fraction / %) Power Scanning rate Remelting (volume fraction) HV
kW mm·min-1
Fe60.3Cr18Mo17B2.5C2.2 4.0 2000 No ~50% 1085.6 [32]
Fe42Cr23Mo10C12B13 2.5 600 No 45% 900 [33]
Fe37.5Cr27.5C12B13Mo10 2.0/1.4 360 Yes > 50% - [34]
Fe45.8Mo24.2Cr14.7Co7.8C3.2B4.3 0.5 600 No 52.8% 1200 [35]
Fe34Co34B20Si5C3Nb4 1.9 3000 No ~90% 1245 [36]
Fe34Co34B20Si5C3Nb4 1.2 1020 No 87.6% 1283 [37]
Fe35.9Co35.9B19Si4.8Nb4.3 1.2 1020 No 80%-90% - [38]
Ni40.8Fe27.2B18Si10Nb4 0.7/3.5 8000 Yes 63% 1200 [39]
(Ni100 - x Fe x )62B18Si18Nb2 5.5/14 8000 Yes 36%-48% > 1200 [40]
Co34Cr29B14Fe8Ni8Si7 0.52 100 No 85.1% - [41]
Co34Cr29B14Fe8Ni8Si7 0.233 100 No 81.15% 1192.5 [42]
Ni39Fe26B18Si10Nb4C3 2.75 2400 No 76.7% 1187 [43]
Fe48.7Cr23.8Mo8.2B9.1C8.2Nb2 4.0 900 No ~50% 1024 [44]
(Fe25Co25Ni25(B0.7Si0.3)25)100 - x Nb x 2.5/3 1200 Yes A little > 800 [45]
Fe25Co25Ni25(B x Si1 - x )25 2.0/1.5 300 Yes - 839 [31]
Fe36Cr32Co14.5Ni10Si4.25B3.25 0.467 100 No 49% - [30]
Fe21.84Cr29Co20.16Ni8Si7B14 0.467 100 No 66.7% 850 [46]
Table 1  Coatings of amorphous/high-entropy amorphous alloys[30-46]
Fig.1  Microstructures of CoCrFeNiSiB coating by laser cladding with different powers[42]
(a) 233 W (b) 476 W (c) 583 W (d) 700 W
Fig.2  SEM images of sectional morphology of the (CoCrFeMnNi)85Ti15 high-entropy alloy (HEA) coating[52]
(a) microstructure in the bottom-middle region
(b) bottom equiaxed dendrites
(c) middle snowflake-like dendrites
Fig.3  SEM images of the polished surface morphology for the high-velocity air fuel (HVAF)-sprayed Fe49.7Cr18Mn1.9Mo7.4W1.6-B15.2C3.8Si2.4 amorphous coating[55]
(a) secondary electron image (b) back scatter electron image
(c) enlargement for the rectangle 1 in Fig.3b (d) enlargement for the rectangle 2 in Fig.3b
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