基体表面喷丸处理对纳米晶涂层循环氧化行为的影响

doi:10.11900/0412.1961.2022.00183

金属学报

2023, Vol. 59

Issue (5): 668-678 DOI: 10.11900/0412.1961.2022.00183

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基体表面喷丸处理对纳米晶涂层循环氧化行为的影响

黄鼎¹, 乔岩欣¹(

), 杨兰兰¹, 王金龙², 陈明辉², 朱圣龙³, 王福会²

¹江苏科技大学材料科学与工程学院镇江 212003
²东北大学沈阳材料科学国家研究中心东北大学联合研究分部沈阳 110819
³中国科学院金属研究所沈阳 110016

Effect of Shot Peening of Substrate Surface on Cyclic Oxidation Behavior of Sputtered Nanocrystalline Coating

HUANG Ding¹, QIAO Yanxin¹(

), YANG Lanlan¹, WANG Jinlong², CHEN Minghui², ZHU Shenglong³, WANG Fuhui²

¹School of Materials Science and Engineering, Jiangsu University of Science and Technology, Zhenjiang 212003, China
²Shenyang National Key Laboratory for Materials Science, Northeastern University, Shenyang 110819, China
³Institute of Metal Research, Chinese Academy of Sciences, Shenyang 110016, China

引用本文:

黄鼎, 乔岩欣, 杨兰兰, 王金龙, 陈明辉, 朱圣龙, 王福会. 基体表面喷丸处理对纳米晶涂层循环氧化行为的影响[J]. 金属学报, 2023, 59(5): 668-678.
Ding HUANG, Yanxin QIAO, Lanlan YANG, Jinlong WANG, Minghui CHEN, Shenglong ZHU, Fuhui WANG. Effect of Shot Peening of Substrate Surface on Cyclic Oxidation Behavior of Sputtered Nanocrystalline Coating[J]. Acta Metall Sin, 2023, 59(5): 668-678.

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摘要:

采用磁控溅射技术分别在抛光和喷丸处理后的镍基单晶高温合金基体上制备纳米晶涂层，并研究了2种涂层在1100℃下的循环氧化行为。采用XRD、SEM和EDS表征涂层的物相组成和微观形貌。结果表明，1100℃下2种纳米晶涂层的循环氧化增重趋势基本一致，均能在表面形成致密的氧化膜，展现出优异的抗氧化性能。2种纳米晶涂层与基体的界面及界面附近区域的微观形貌演变有所差异，随着氧化实验的进行，在抛光基体/涂层界面处涂层一侧观察到γ'相的持续形成；在喷丸基体/涂层界面处涂层一侧未发现此现象，而在基体一侧观察到γ'相不断长大。

关键词 ：喷丸处理, 纳米晶涂层, 循环氧化, 磁控溅射

Abstract：

In addition to changing the surface roughness of the superalloy, the substrate surface treatment can also modify the microstructure of the surface, which affects the high-temperature oxidation behavior of the high-temperature protective coating. However, there are few reports about the effect of superalloy surface treatment on the oxidation behavior of nanocrystalline coatings. In this work, nanocrystalline coatings were sputtered on the nickel-based single crystal superalloy after two different surface treatments of polishing and shot peening, and their cyclic oxidation behavior at 1100^oC was investigated. The phase composition and microstructure of nanocrystalline coatings were characterized by SEM, XRD, and EDS. The results indicated that the cyclic oxidation kinetics of both nanocrystalline coatings at 1100^oC were similar. A dense oxide film could be formed on the surface of nanocrystalline coatings, showing excellent oxidation resistance. However, the microstructure evolution of the interface between the nanocrystalline coating and shot-peened superalloy substrate differed from that between the nanocrystalline coating and polished superalloy substrate. The sustained formation of the γ′ phase in the nanocrystalline coating near the polished substrate/coating interface was observed during high-temperature oxidation. This phenomenon was not found at the nanocrystalline coating near the shot peened substrate/coating interface, while the continuous growth of the γ' phase was observed at the substrate.

Key words： shot peening nanocrystalline coating cyclic oxidation magnetron sputtering

收稿日期: 2022-04-19

ZTFLH:

TG172

基金资助:国家自然科学基金项目(51801021);国家自然科学基金项目(52001142);工业和信息技术部项目(MJ-2017-J-99);教育部中央高效基本科研业务费项目(N2102015)

作者简介: 黄鼎，男，1996年生，硕士生

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https://www.ams.org.cn/CN/10.11900/0412.1961.2022.00183 或 https://www.ams.org.cn/CN/Y2023/V59/I5/668

图1 沉积在抛光和喷丸N5单晶高温合金表面上的纳米晶涂层的截面和表面形貌

图2 纳米晶涂层1100℃循环氧化动力学曲线和单位面积的质量增重(ΔM)与氧化时间(t)的拟合曲线

图3 1100℃下纳米晶涂层在不同循环次数后的XRD谱

图4 沉积在抛光和喷丸高温合金表面上的纳米晶涂层在1100℃下100 cyc后的截面和表面形貌

图5 1100℃下氧化0、5、20和100 cyc后抛光高温合金基体/纳米晶涂层界面微观组织及沿虚线的EDS线扫描结果

图6 1100℃下氧化0、5、20和100 cyc后喷丸高温合金基体/纳米晶涂层界面微观组织及沿虚线的EDS线扫描结果

表1 图5d和6d中点1~4的EDS结果 (mass fraction / %)

图7 沉积在抛光和喷丸高温合金表面上的纳米晶涂层在1100℃下20和100 cyc后的截面微观组织

表2 图7点1~8处Al元素的EDS结果

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